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It was found that linear poly glycerol monomethacrylate —poly 2-hydroxypropyl methacrylate PGMA—PHPMA diblock copolymer spheres and worms do not survive the high shear homogenisation conditions used for emulsification. Stable emulsions are obtained, but the copolymer acts as a polymeric surfactant; individual chains rather than particles are adsorbed at the oil—water interface. Particle dissociation during emulsification is attributed to the weakly hydrophobic character of the PHPMA block. TEM studies confirm that the resulting cross-linked spherical or worm-like nanoparticles survive emulsification and produce genuine Pickering emulsions.
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